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BA Comair and SAA operate 1-stop flights from Cape Town to Victoria Falls via Johannesburg. It's about 7 hours of travelling time if you can wangle a 3-hour stopover at O.R. Tambo International Airport.
There are 4 main routes to drive from Cape Town to Victoria Falls:
The shortest route is on the N1 and N12 via Gaborone, which takes about 30 hours and is some 2377km.
Driving the N1 via Johannesburg and then the N11 into Botswana, also takes about 30 hours driving, but is 2598km.
Driving the N1 all the way through South African and then going through Zimbabwe via Bulawayo, takes about 32 hours and is some 2698km.
Along the N7 towards Windhoek, and then onwards to Victoria Falls via Katima Mulilo.
The Intercape bus offers coach trips from Cape Town to Vic Falls via Windhoek.